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An overview of the current status of the development of a nuclear clock based on the state of lowest known nuclear excitation energy in 229Th is presented. The text is especially written for the interested reader without any particular knowledge in this field of research. It is thus ideal as an introductory reading to get a broad overview of the various different aspects of the field; in addition, it can serve as a guideline for future research. An introductory part is provided, giving a historic context and explaining the fundamental concept of clocks. Finally, potential candidates for nuclear clocks other than 229Th are discussed.

Nuclear resonant excitation and detection of its decay signal for the 26.27-keV level of Hg201 is demonstrated with high-brilliance synchrotron radiation (SR) and a fast x-ray detector system. This SR-based photonuclear excitation scheme, known as nuclear resonant scattering (NRS) in the field of materials science, is also useful for investigating nuclear properties, such as the half-lives and radiative widths of excited nuclear levels. To date, because of the limited time response of the x-ray detector, the nuclear levels to which this method could be applied have been limited to the one whose half-lives are longer than ∼1 ns. The faster time response of the NRS measurement makes possible NRS experiments on nuclear levels with much shorter half-lives. We have fabricated an x-ray detector system that has a time resolution of 56 ps and a shorter tail function than that reported previously. With the implemented detector system, the NRS signal of the 26.27-keV state of Hg201 could be clearly discriminated from the electronic scattering signal at an elapsed time of 1 ns after the SR pulse. The half-life of the state was determined as 629 ± 18 ps, which has better precision by a factor of three compared with that reported to date obtained from nuclear decay spectroscopy

We report on the pulse compression of an 18.5 MHz repetition rate pulse train from 230 fs to sub-40 fs by nonlinear spectral broadening in a multi-pass cell and subsequent chirp removal. The compressed pulse energy is 4.5 μJ, which corresponds to 84 W of average power, with a compression efficiency of 88%. This recently introduced compression scheme is suitable for a large pulse energy range and for high average power. In this paper, we show that it can achieve three times shorter pulses than previously demonstrated.

Direct laser excitation of the lowest known nuclear excited state in $229\mathrm{Th}$ has been a long-standing objective. It is generally assumed that reaching this goal would require a considerably reduced uncertainty of the isomer’s excitation energy compared to the presently adopted value of $(7.8\pm 0.5)\mathrm{eV}$. Here we present a direct laser excitation scheme for $229m\mathrm{Th}$, which circumvents this requirement. The proposed excitation scheme makes use of already existing laser technology and therefore paves the way for nuclear laser spectroscopy. In this concept, the recently experimentally observed internal-conversion decay channel of the isomeric state is used for probing the isomeric population. A signal-to-background ratio of better than $10^4$ and a total measurement time of less than three days for laser scanning appear to be achievable.

The isotope 229Th is the only nucleus known to possess an excited state 229mTh in the energy range of a few electron volts, a transition energy typical for electrons in the valence shell of atoms, but about four orders of magnitude lower than common nuclear excitation energies. A number of applications of this unique nuclear system, which is accessible by optical methods, have been proposed. Most promising among them appears a highly precise nuclear clock that outperforms existing atomic timekeepers. Here we present the laser spectroscopic investigation of the hyperfine structure of 229mTh2+, yielding values of fundamental nuclear properties, namely the magnetic dipole and electric quadrupole moments as well as the nuclear charge radius. After the recent direct detection of this long-searched-for isomer, our results now provide detailed insight into its nuclear structure and present a method for its non-destructive optical detection, an important step towards the development of a nuclear clock.

An alternative method to determine the excitation energy of the 229mTh isomer via the laser-induced electronic bridge is investigated theoretically. In the presence of an optical or ultra-violet laser at energies that fulfill a two-photon resonance condition, the excited nuclear state can decay by transfering its energy to the electronic shell. A bound electron is then promoted to an excited state by absorption of a laser photon and simultaneous de-excitation of the nucleus. We present calculated rates for the laser-induced electronic bridge process and discuss the experimental requirements for the corresponding setup. Our results show that depending on the actual value of the nuclear transition energy, the rate can be very high, with an enhancement factor compared to the radiative nuclear decay of up to 10^8.

We demonstrate nonlinear pulse compression by multi-pass cell spectral broadening (MPCSB) from 860 fs to 115 fs with compressed pulse energy of 7.5 μJ, average power of 300 W and close to diffraction-limited beam quality. The transmission of the compression unit is >90%. The results show that this recently introduced  compression scheme for peak powers above the threshold for catastrophic self-focusing can be scaled to smaller pulse energies and can achieve a larger compression factor than previously reported. Good homogeneity of the spectral broadening across the beam profile is verified, which distinguishes MPCSB among other bulk compression schemes.

This study sets out to explore the perception of noise, as well as the recovery of meaning or information that it might contain, in arts, science, and daily life. It is realized as an installation based on an arrangement of nitinol drums that create a sonic environment evolving in time and space. The nitinol drums are driven by digital random noise. The observer is free to explore the sonic environment, and will discover regions in time and space with a “meaningful” signal. This discovery of a clear signal in a noisy background holds strong analogies to the scientific search for a nuclear resonance performed in the nuClock project.

With an expected energy of 7.8(5) eV, the isomeric first excited state in Th-229 exhibits the lowest excitation energy of all known nuclei. Until today, a value for the excitation energy has been inferred only by indirect measurements. In this paper, we propose to use the internal conversion decay channel as a probe for the ground-state transition energy. MatLab-based Monte Carlo simulations have been performed to obtain an estimate of the expected statistics and to test the feasibility of the experiment. From the simulations we conclude, that with the presented methods an energy determination with a precision of better than 0.1 eV is possible.